Abstract
We develop an understanding of the anomalous metal state of the parent compounds of recently discovered iron-based superconductors starting from a strong-coupling viewpoint, including orbital degrees of freedom. On the basis of an intermediate-spin (S=1) state for the Fe2+ ions, we derive a Kugel-Khomskii spin-orbital Hamiltonian for the active t(2g) orbitals. It turns out to be a highly complex model with frustrated spin and orbital interactions. We compute its classical phase diagrams and provide an understanding for the stability of the various phases by investigating its spin-only and orbital-only limits. The experimentally observed spin-stripe state is found to be stable over a wide regime of physical parameters and can be accompanied by three different types of orbital orders. Of these the orbital-ferro and orbital-stripe orders are particularly interesting since they break the in-plane lattice symmetry-a robust feature of the undoped compounds. We compute the magnetic excitation spectra for the effective spin Hamiltonian, observing a strong reduction in the ordered moment, and point out that the proposed orbital ordering pattern can be measured in resonant x-ray diffraction.
| Original language | English |
|---|---|
| Pages (from-to) | 054504 |
| Number of pages | 15 |
| Journal | Physical Review. B, Condensed matter and materials physics |
| Volume | 79 |
| Issue number | 5 |
| DOIs | |
| Publication status | Published - Feb 2009 |
Keywords
- DOUBLE EXCHANGE
- MAGNETIC ORDER
- 43 K
- TRANSITION
- FLUCTUATIONS
- LAO1-XFXFEAS
- COMPOUND
- CHARGE
Fingerprint
Dive into the research topics of 'Spin-orbital frustrations and anomalous metallic state in iron-pnictide superconductors'. Together they form a unique fingerprint.Cite this
- APA
- Author
- BIBTEX
- Harvard
- Standard
- RIS
- Vancouver