Organic polariton lasing and the weak- to strong-coupling crossover

Artem Strashko; Peter Kirton; Jonathan Keeling

doi:10.1103/PhysRevLett.121.193601

Organic polariton lasing and the weak- to strong-coupling crossover

Artem Strashko, Peter Kirton, Jonathan Keeling

Research output: Contribution to journal › Article › peer-review

Abstract

Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.

Original language	English
Article number	193601
Number of pages	6
Journal	Physical Review Letters
Volume	121
Issue number	19
DOIs	https://doi.org/10.1103/PhysRevLett.121.193601
Publication status	Published - 9 Nov 2018

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10.1103/PhysRevLett.121.193601

organic_sc_lasing
© 2018, American Physical Society. This work has been made available online in accordance with the publisher’s policies. This is the author created accepted version manuscript following peer review and as such may differ slightly from the final published version. The final published version of this work is available at https://doi.org/10.1103/PhysRevLett.121.193601
Accepted author manuscript, 1.86 MB

Hybrid Polaritonics: Hybrid Polaritonics
Samuel, I. D. W. (PI), Höfling, S. (CoI), Keeling, J. M. J. (CoI) & Turnbull, G. (CoI)
EPSRC
1/09/15 → 31/08/20
Project: Standard
Understand Bose-Einstein Conden of Light: Understanding Bose-Einstein condensation of Light
Kirton, P. G. (PI)
EPSRC
1/01/15 → 31/12/17
Project: Fellowship
CM DTC 2014 - 2022: EPSRC centre for doctoral training in condensed matter physics: Renewal of the CM-DTC
King, P. (PI)
EPSRC
1/08/14 → 31/01/24
Project: Standard

Jonathan Mark James Keeling
- jmjkst-andrews.acuk
- School of Physics and Astronomy - Head of the School of Physics and Astronomy, Professor
- Centre for Designer Quantum Materials
- Condensed Matter Physics
Person: Academic

Data underpinning: Organic polariton lasing and the weak- to strong-coupling crossover
Strashko, A. (Creator), Kirton, P. G. (Creator) & Keeling, J. M. J. (Creator), University of St Andrews, 2018
DOI: 10.17630/3fbfe834-d0e1-4e21-96f2-7afcf1c261ba
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title = "Organic polariton lasing and the weak- to strong-coupling crossover",

abstract = "Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers. ",

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AU - Kirton, Peter

AU - Keeling, Jonathan

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AB - Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.

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DO - 10.1103/PhysRevLett.121.193601

M3 - Article

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VL - 121

JO - Physical Review Letters

JF - Physical Review Letters

IS - 19

M1 - 193601

ER -

Organic polariton lasing and the weak- to strong-coupling crossover

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Projects

Hybrid Polaritonics: Hybrid Polaritonics

Understand Bose-Einstein Conden of Light: Understanding Bose-Einstein condensation of Light

CM DTC 2014 - 2022: EPSRC centre for doctoral training in condensed matter physics: Renewal of the CM-DTC

Profiles

Jonathan Mark James Keeling

Datasets

Data underpinning: Organic polariton lasing and the weak- to strong-coupling crossover

Cite this