Multimode organic polariton lasing

Kristin B. Arnardottir; Antti J. Moilanen; Artem Strashko; Päivi Törmä; Jonathan Keeling

doi:10.1103/PhysRevLett.125.233603

Multimode organic polariton lasing

Kristin B. Arnardottir, Antti J. Moilanen, Artem Strashko, Päivi Törmä, Jonathan Keeling

Research output: Contribution to journal › Article › peer-review

Abstract

We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of nonlasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and nonlasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.

Original language	English
Article number	233603
Number of pages	7
Journal	Physical Review Letters
Volume	125
Issue number	23
Early online date	2 Dec 2020
DOIs	https://doi.org/10.1103/PhysRevLett.125.233603
Publication status	Published - 4 Dec 2020

Access to Document

10.1103/PhysRevLett.125.233603

Arnardottir-2020-Multimode-organic-PhysRevLett-125-233603
Copyright © 2020 American Physical Society. This work has been made available online in accordance with publisher policies or with permission. Permission for further reuse of this content should be sought from the publisher or the rights holder. This is the final published version of the work, which was originally published at https://doi.org/10.1103/PhysRevLett.125.233603.
Final published version, 539 KB

Cite this

@article{71230b23e41a4b2985cd54c46693b9b6,

title = "Multimode organic polariton lasing",

abstract = "We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of nonlasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and nonlasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.",

author = "Arnardottir, {Kristin B.} and Moilanen, {Antti J.} and Artem Strashko and P{\"a}ivi T{\"o}rm{\"a} and Jonathan Keeling",

note = "Funding: KBA and JK acknowledge financial support from EPSRC program “Hybrid Polaritonics” (EP/M025330/1). AJM and PT acknowledge support by the Academy of Finland under project numbers 303351, 307419, 327293, 318987 (QuantERA project RouTe) and 318937 (PROFI), and by Centre for Quantum Engineering (CQE) at Aalto University. AJM acknowledges financial support by the Jenny and Antti Wihuri Foundation. AS acknowledges support from the EPSRC CM-CDT (EP/L015110/1).",

year = "2020",

month = dec,

day = "4",

doi = "10.1103/PhysRevLett.125.233603",

language = "English",

volume = "125",

journal = "Physical Review Letters",

issn = "0031-9007",

publisher = "American Physical Society",

number = "23",

}

TY - JOUR

T1 - Multimode organic polariton lasing

AU - Arnardottir, Kristin B.

AU - Moilanen, Antti J.

AU - Strashko, Artem

AU - Törmä, Päivi

AU - Keeling, Jonathan

N1 - Funding: KBA and JK acknowledge financial support from EPSRC program “Hybrid Polaritonics” (EP/M025330/1). AJM and PT acknowledge support by the Academy of Finland under project numbers 303351, 307419, 327293, 318987 (QuantERA project RouTe) and 318937 (PROFI), and by Centre for Quantum Engineering (CQE) at Aalto University. AJM acknowledges financial support by the Jenny and Antti Wihuri Foundation. AS acknowledges support from the EPSRC CM-CDT (EP/L015110/1).

PY - 2020/12/4

Y1 - 2020/12/4

N2 - We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of nonlasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and nonlasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.

AB - We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of nonlasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and nonlasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.

UR - https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.125.233603

U2 - 10.1103/PhysRevLett.125.233603

DO - 10.1103/PhysRevLett.125.233603

M3 - Article

SN - 0031-9007

VL - 125

JO - Physical Review Letters

JF - Physical Review Letters

IS - 23

M1 - 233603

ER -

Multimode organic polariton lasing

Abstract

Access to Document

Other files and links

Fingerprint

Hybrid Polaritonics: Hybrid Polaritonics

Data Underpinning: Multimode Organic Polariton Lasing

Cite this

Multimode organic polariton lasing

Abstract

Access to Document

Other files and links

Fingerprint

Projects

Hybrid Polaritonics: Hybrid Polaritonics

Datasets

Data Underpinning: Multimode Organic Polariton Lasing

Cite this