Magnetic-field tunable intertwined checkerboard charge order and nematicity in the surface layer of Sr2RuO4

Carolina A. Marques, Luke Charles Rhodes, Rosalba Fittipaldi, Veronica Granata, Chi Ming Yim, Renato Buzio, Andrea Gerbi, Antonio Vecchione, Andreas W. Rost, Peter Wahl*

*Corresponding author for this work

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Abstract

In strongly correlated electron materials, the electronic, spin, and charge degrees of freedom are closely intertwined. This often leads to the stabilization of emergent orders that are highly sensitive to external physical stimuli promising opportunities for technological applications. In perovskite ruthenates, this sensitivity manifests in dramatic changes of the physical properties with subtle structural details of the RuO6 octahedra, stabilizing enigmatic correlated ground states, from a hotly debated superconducting state via electronic nematicity and metamagnetic quantum criticality to ferromagnetism. Here, it is demonstrated that the rotation of the RuO6 octahedra in the surface layer of Sr2RuO4 generates new emergent orders not observed in the bulk material. Through atomic-scale spectroscopic characterization of the low-energy electronic states, four van Hove singularities are identified in the vicinity of the Fermi energy. The singularities can be directly linked to intertwined nematic and checkerboard charge order. Tuning of one of these van Hove singularities by magnetic field is demonstrated, suggesting that the surface layer undergoes a Lifshitz transition at a magnetic field of ≈32T. The results establish the surface layer of Sr2RuO4 as an exciting 2D correlated electron system and highlight the opportunities for engineering the low-energy electronic states in these systems.
Original languageEnglish
Article number2100593
Number of pages8
JournalAdvanced Materials
Volume33
Issue number32
Early online date27 Jun 2021
DOIs
Publication statusPublished - 12 Aug 2021

Keywords

  • Electronic structure
  • Ruthenate perovskites
  • Strongly correlated electron systems
  • Quantum criticality

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