Local tuning of Rydberg exciton energies in nanofabricated Cu2O pillars

Anindya Sundar Paul, Sai Kiran Rajendran*, D Ziemkiewicz, T Volz, Hamid Ohadi*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

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Abstract

Rydberg excitons in Cu2O feature giant optical nonlinearities. To exploit these nonlinearities for quantum applications, the confinement must match the Rydberg blockade size, which in Cu2O could be as large as a few microns. Here, in a top-down approach, we show how exciton confinement can be realised by focused-ion-beam etching of a polished bulk Cu2O crystal without noticeable degradation of the excitonic properties. The etching of the crystal to micron sizes allows for tuning the energies of Rydberg excitons locally, and precisely, by optically induced temperature change. These results pave the way for exploiting the large nonlinearities of Rydberg excitons in micropillars for making non-classical light sources, while the precise tuning of their emission energy opens up a viable pathway for realizing a scalable photonic quantum simulation platform.
Original languageEnglish
Article number43
Number of pages8
JournalCommunications Materials
Volume5
Issue number43
DOIs
Publication statusPublished - 28 Mar 2024

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