TY - JOUR
T1 - Fermi surface of PtCoO2 from quantum oscillations and electronic structure calculations
AU - Arnold, F.
AU - Naumann, M.
AU - Rosner, H.
AU - Kikugawa, N.
AU - Graf, D.
AU - Balicas, L.
AU - Terashima, T.
AU - Uji, S.
AU - Takatsu, H.
AU - Khim, S.
AU - Mackenzie, A. P.
AU - Hassinger, E.
N1 - The authors would like to acknowledge the financial support from the Max-Planck Society. E.H. and M.N. acknowledge support from Deutsche Forschungsgemeinschaft (DFG) through the Project No. 107745057 (TRR80: From Electronic Correlations to Functionality). This work is also supported by JSPS KAKENHI (No. 18K04715). A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by the National Science Foundation Cooperative Agreements No. DMR-1157490 and No. DMR-1644779 and the State of Florida.
PY - 2020/5/1
Y1 - 2020/5/1
N2 - The delafossite series of layered oxides includes some of the highest conductivity metals ever discovered. Of these, PtCoO2, with a room-temperature resistivity of 1.8 μΩcm for in-plane transport, is the most conducting of all. The high conduction takes place in triangular lattice Pt layers, separated by layers of Co-O octahedra, and the electronic structure is determined by the interplay of the two types of layers. We present a detailed study of quantum oscillations in PtCoO2, at temperatures down to 35 mK and magnetic fields up to 30 T. As for PdCoO2 and PdRhO2, the Fermi surface consists of a single cylinder with mainly Pt character and an effective mass close to the free-electron value. Due to Fermi-surface warping, two close-lying high frequencies are observed. Additionally, a pronounced difference frequency appears. By analyzing the detailed angular dependence of the quantum-oscillation frequencies, we establish the warping parameters of the Fermi surface. We compare these results to the predictions of first-principles electronic-structure calculations including spin-orbit coupling on Pt and Co and on-site correlation U on Co, and hence demonstrate that electronic correlations in the Co-O layers play an important role in determining characteristic features of the electronic structure of PtCoO2.
AB - The delafossite series of layered oxides includes some of the highest conductivity metals ever discovered. Of these, PtCoO2, with a room-temperature resistivity of 1.8 μΩcm for in-plane transport, is the most conducting of all. The high conduction takes place in triangular lattice Pt layers, separated by layers of Co-O octahedra, and the electronic structure is determined by the interplay of the two types of layers. We present a detailed study of quantum oscillations in PtCoO2, at temperatures down to 35 mK and magnetic fields up to 30 T. As for PdCoO2 and PdRhO2, the Fermi surface consists of a single cylinder with mainly Pt character and an effective mass close to the free-electron value. Due to Fermi-surface warping, two close-lying high frequencies are observed. Additionally, a pronounced difference frequency appears. By analyzing the detailed angular dependence of the quantum-oscillation frequencies, we establish the warping parameters of the Fermi surface. We compare these results to the predictions of first-principles electronic-structure calculations including spin-orbit coupling on Pt and Co and on-site correlation U on Co, and hence demonstrate that electronic correlations in the Co-O layers play an important role in determining characteristic features of the electronic structure of PtCoO2.
UR - https://www.scopus.com/pages/publications/85086001461
U2 - 10.1103/PhysRevB.101.195101
DO - 10.1103/PhysRevB.101.195101
M3 - Article
SN - 1098-0121
VL - 101
JO - Physical Review B
JF - Physical Review B
IS - 19
M1 - 195101
ER -