Expansion of the ADOR strategy for the synthesis of new zeolites: the synthesis of IPC-12 from zeolite UOV

Valeryia Kasneryk; Mariya Shamzhy; Maksym Opanasenko; Paul S. Wheatley; Samuel A. Morris; Samantha E. Russell; Alvaro Mayoral; Michal Trachta; Jiří Čejka; Russell E. Morris

doi:10.1002/anie.201700590

Expansion of the ADOR strategy for the synthesis of new zeolites: the synthesis of IPC-12 from zeolite UOV

Valeryia Kasneryk, Mariya Shamzhy, Maksym Opanasenko, Paul S. Wheatley, Samuel A. Morris, Samantha E. Russell, Alvaro Mayoral, Michal Trachta, Jiří Čejka, Russell E. Morris

Research output: Contribution to journal › Article › peer-review

Abstract

The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.

Original language	English
Pages (from-to)	4324-4327
Number of pages	5
Journal	Angewandte Chemie
Volume	56
Issue number	15
Early online date	13 Mar 2017
DOIs	https://doi.org/10.1002/anie.201700590
Publication status	Published - 3 Apr 2017

Keywords

ADOR
Germanosilicates
Isoreticular materials
Structure rearrangement
Zeolites

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10.1002/anie.201700590Licence: CC BY

Kasneryk_et_al-2017-Angewandte_Chemie_International_CC
Copyright 2017 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
Final published version, 1.28 MBLicence: CC BY

CRITICAT CDT: Critical Resource Catalysis - CRITICAT
Smith, A. D. (PI), Nolan, S. P. (CoI) & Westwood, N. J. (CoI)
EPSRC
1/05/14 → 31/10/22
Project: Standard
Assembly Disassembly Reassembly: Assembly disassembly reassembly - New routes to extended structures and their impact
Morris, R. E. (PI)
EPSRC
1/08/13 → 31/07/18
Project: Fellowship
Hemilabile switchable metal-organic: Hemilabile and switchable metal-organic frameworks
Morris, R. E. (PI)
EPSRC
1/03/13 → 28/02/16
Project: Standard

Russell Edward Morris, FRS FRSE FRSC FLSW
- rem1st-andrews.acuk
- School of Chemistry - Bishop Wardlaw Professor
- EaSTCHEM
Person: Academic

Data underpinning "Expansion of the ADOR strategy for the synthesis of new zeolites: The synthesis of IPC-12 from zeolite UOV"
Kasneryk, V. (Creator), Shamzh, M. (Creator), Opanasenko, M. (Creator), Wheatley, P. S. (Creator), Morris, S. A. (Creator), Russell, S. (Creator), Mayoral, A. (Creator), Trachta, M. (Creator), Čejka, J. (Creator) & Morris, R. E. (Creator), University of St Andrews, 2019
DOI: 10.17630/4d5783d8-493d-43f4-abd9-39cf20c3dcf5
Dataset

Cite this

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title = "Expansion of the ADOR strategy for the synthesis of new zeolites: the synthesis of IPC-12 from zeolite UOV",

abstract = "The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.",

keywords = "ADOR, Germanosilicates, Isoreticular materials, Structure rearrangement, Zeolites",

author = "Valeryia Kasneryk and Mariya Shamzhy and Maksym Opanasenko and Wheatley, {Paul S.} and Morris, {Samuel A.} and Russell, {Samantha E.} and Alvaro Mayoral and Michal Trachta and Ji{\v r}{\'i} {\v C}ejka and Morris, {Russell E.}",

note = "R.E.M. thanks the Royal Society and the Engineering and Physical Sciences Research Council (Grants EP/K025112/1, EP/K005499/1, EP/L016419/1) for funding work in this area and for providing a Ph.D. studentship to S.E.R. through the Criticat Centre for Doctoral training. R.E.M. and M. O. acknowledge the OP VVV {"}Excellent Research Teams{"}, project No. CZ.02.1.01/0.0/0.0/15_003/0000417 - CUCAM. J.{\v C}., V.K., and M.T. acknowledge the Czech Science Foundation for the project of the Centre of Excellence (P106/12/G015) and J.{\v C} has received funding from the European Union's Horizon2020 research and innovation programme under grant agreement No 640979. The research leading to these results has received funding from the European Union Seventh Framework Programme under Grant Agreement No. 312483—ESTEEM2 (Integrated Infrastructure Initiative–I3).",

year = "2017",

month = apr,

day = "3",

doi = "10.1002/anie.201700590",

language = "English",

volume = "56",

pages = "4324--4327",

journal = "Angewandte Chemie",

issn = "0044-8249",

publisher = "John Wiley & Sons, Ltd",

number = "15",

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TY - JOUR

T1 - Expansion of the ADOR strategy for the synthesis of new zeolites

T2 - the synthesis of IPC-12 from zeolite UOV

AU - Kasneryk, Valeryia

AU - Shamzhy, Mariya

AU - Opanasenko, Maksym

AU - Wheatley, Paul S.

AU - Morris, Samuel A.

AU - Russell, Samantha E.

AU - Mayoral, Alvaro

AU - Trachta, Michal

AU - Čejka, Jiří

AU - Morris, Russell E.

N1 - R.E.M. thanks the Royal Society and the Engineering and Physical Sciences Research Council (Grants EP/K025112/1, EP/K005499/1, EP/L016419/1) for funding work in this area and for providing a Ph.D. studentship to S.E.R. through the Criticat Centre for Doctoral training. R.E.M. and M. O. acknowledge the OP VVV "Excellent Research Teams", project No. CZ.02.1.01/0.0/0.0/15_003/0000417 - CUCAM. J.Č., V.K., and M.T. acknowledge the Czech Science Foundation for the project of the Centre of Excellence (P106/12/G015) and J.Č has received funding from the European Union's Horizon2020 research and innovation programme under grant agreement No 640979. The research leading to these results has received funding from the European Union Seventh Framework Programme under Grant Agreement No. 312483—ESTEEM2 (Integrated Infrastructure Initiative–I3).

PY - 2017/4/3

Y1 - 2017/4/3

N2 - The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.

AB - The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.

KW - ADOR

KW - Germanosilicates

KW - Isoreticular materials

KW - Structure rearrangement

KW - Zeolites

U2 - 10.1002/anie.201700590

DO - 10.1002/anie.201700590

M3 - Article

SN - 0044-8249

VL - 56

SP - 4324

EP - 4327

JO - Angewandte Chemie

JF - Angewandte Chemie

IS - 15

ER -

Expansion of the ADOR strategy for the synthesis of new zeolites: the synthesis of IPC-12 from zeolite UOV

Abstract

Keywords

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Projects

CRITICAT CDT: Critical Resource Catalysis - CRITICAT

Assembly Disassembly Reassembly: Assembly disassembly reassembly - New routes to extended structures and their impact

Hemilabile switchable metal-organic: Hemilabile and switchable metal-organic frameworks

Profiles

Russell Edward Morris, FRS FRSE FRSC FLSW

Datasets

Data underpinning "Expansion of the ADOR strategy for the synthesis of new zeolites: The synthesis of IPC-12 from zeolite UOV"

Cite this