Abstract
Correlations between magnetism and morphology of iron nanostructures of monatomic height on Pt(997) substrates are studied using x-ray magnetic circular dichroism as well as scanning tunneling microscopy and helium scattering. A drastic collapse of the average magnetization by more than a factor of 4 is observed when increasing the iron coverage from 0.1 to 0.2 ML. This effect goes along with a softening of the magnetic anisotropy energy and a gradual reorientation of the magnetic easy axis from in plane to out of plane. The experimental findings together with electronic density-functional calculations suggest the formation of a complex magnetic phase in corrugated rim regions of Fe islands, leading to both ferromagnetic and antiferromagnetic exchange couplings of Fe moments depending on their various local bonding configurations.
| Original language | English |
|---|---|
| Article number | 104430 |
| Pages (from-to) | - |
| Number of pages | 7 |
| Journal | Physical Review. B, Condensed matter and materials physics |
| Volume | 79 |
| Issue number | 10 |
| DOIs | |
| Publication status | Published - Mar 2009 |
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