TY - JOUR
T1 - Absorption, photoluminescence, and resonant Rayleigh scattering probes of condensed microcavity polaritons
AU - Marchetti, F. M.
AU - Keeling, Jonathan Mark James
AU - Szymanska, M. H.
AU - Littlewood, P. B.
PY - 2007/9
Y1 - 2007/9
N2 - We investigate and compare different optical probes of a condensed state of microcavity polaritons in expected experimental conditions of nonresonant pumping. We show that the energy- and momentum-resolved resonant Rayleigh signal provides a distinctive probe of condensation as compared to, e.g., photoluminescence emission. In particular, the presence of a collective sound mode both above and below the chemical potential can be observed, as well as features directly related to the density of states of particle-hole-like excitations. Both resonant Rayleigh response and the absorption and photoluminescence are affected by the presence of quantum well disorder, which introduces a distribution of oscillator strengths between quantum well excitons at a given energy and cavity photons at a given momentum. As we show, this distribution makes it important that in the condensed regime, scattering by disorder is taken into account to all orders. We show that, in the low-density linear limit, this approach correctly describes inhomogeneous broadening of polaritons. In addition, in this limit, we extract a linear blueshift of the lower polariton versus density, with a coefficient determined by temperature and by a characteristic disorder length.
AB - We investigate and compare different optical probes of a condensed state of microcavity polaritons in expected experimental conditions of nonresonant pumping. We show that the energy- and momentum-resolved resonant Rayleigh signal provides a distinctive probe of condensation as compared to, e.g., photoluminescence emission. In particular, the presence of a collective sound mode both above and below the chemical potential can be observed, as well as features directly related to the density of states of particle-hole-like excitations. Both resonant Rayleigh response and the absorption and photoluminescence are affected by the presence of quantum well disorder, which introduces a distribution of oscillator strengths between quantum well excitons at a given energy and cavity photons at a given momentum. As we show, this distribution makes it important that in the condensed regime, scattering by disorder is taken into account to all orders. We show that, in the low-density linear limit, this approach correctly describes inhomogeneous broadening of polaritons. In addition, in this limit, we extract a linear blueshift of the lower polariton versus density, with a coefficient determined by temperature and by a characteristic disorder length.
KW - BOSE-EINSTEIN CONDENSATION
KW - COUPLED QUANTUM-WELLS
KW - SEMICONDUCTOR MICROCAVITIES
KW - EXCITON POLARITONS
KW - AMPLIFIER
KW - DYNAMICS
KW - DISORDER
KW - RELAXATION
KW - BOTTLENECK
KW - LINEWIDTH
UR - http://www.scopus.com/inward/record.url?scp=34648843542&partnerID=8YFLogxK
U2 - 10.1103/PhysRevB.76.115326
DO - 10.1103/PhysRevB.76.115326
M3 - Article
SN - 1098-0121
VL - 76
SP - 115326
JO - Physical Review. B, Condensed matter and materials physics
JF - Physical Review. B, Condensed matter and materials physics
IS - 11
ER -